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Effect of Catalyst Coating Strategy on NOx Reduction and Passive Soot Oxidation for Selective Catalytic Oxidation-Selective Catalytic Reduction Catalyst on Diesel Particulate Filter Tongji University

SAE Technical Papers (1906-current) Available online

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Format:
Book
Conference/Event
Author/Creator:
Chen, Ying-jie, author.
Contributor:
Hu, Zhiyuan
Lou, Diming
Tan, Piqiang
Yang, Wenming
Yao, Chaojie
Conference Name:
WCX SAE World Congress Experience (2025-04-08 : Detroit, Michigan, United States)
Language:
English
Physical Description:
1 online resource cm
Place of Publication:
Warrendale, PA SAE International 2025
Summary:
Selective catalytic oxidation/reduction catalysts coated on diesel particulate filters (SDPF) are an important technology route to meet next-stage emission regulations. The previous research of the research group showed that compared with SDPF coated with Cu-SSZ-13, the SDPF coated with novel selective catalytic oxidation-selective catalytic reduction (SCO-SCR) catalyst, which combined MnO2-CeO2/Al2O3 and Cu-SSZ-13, can simultaneously improve NOx reduction and soot oxidation performance. Catalyst coating strategy is an important parameter affecting the performance of SDPF. In this study, the effects of different coating strategies of SCO-SCR catalysts (C25, C50, C75, and C100) on the performance of NOx reduction and soot oxidation in SDPF were investigated. The results show that, as the inlet gas temperature increases, NO emissions first decrease and then increase, NOx conversion efficiency first increases and then decreases, and the rich-NO2 area, NH3 oxidation rate, N2O, CO, CO2 emissions, and pressure drop increase. By expanding the catalyst coating area, the NH3 oxidation rate, NOx conversion efficiency, NO2, N2O, CO, CO2 emission and pressure drop of filter wall all increased, the pressure drop of soot cake layer and NO emissions decreased. When the temperature is 450 °C, there are rich-NO2 areas at both the front end and rear end of C100. The 25% area at the rear end of the filter wall coated with SCO-SCR catalyst can increase NOx conversion efficiency and soot regeneration efficiency. While the impact on N2O generation is small. Still, it will lead to excessive NO2 emissions. The increased magnitude in NOx conversion efficiency and soot regeneration efficiency decease as the catalyst coating area expands
Notes:
Vendor supplied data
Publisher Number:
2025-01-8490
Access Restriction:
Restricted for use by site license

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