Optical multidimensional coherent spectroscopy / Hebin Li [and four others].

Format:

Book

Author/Creator:

Li, Hebin, author.

Language:

English

Subjects (All):

Chemistry.

Optical spectroscopy.

Science.

Physical Description:

1 online resource (305 pages)

Place of Publication:

Oxford, England : Oxford University Press, [2023]

Summary:

Aimed at post-doctoral scientists, researchers, and graduate students in physics, this book provides an introduction to optical multidimensional coherent spectroscopy, a relatively new method of studying materials based on using ultrashort light pulses to perform spectroscopy.

Contents:

cover

titlepage

copyright

dedication

preface

Acknowledgements

Table of symbols

Table of acronyms

contents

Basics of ultrafast spectroscopy

Basics of spectroscopy: linear versus nonlinear

Ultrashort pulses

Ultrafast nonlinear/coherent spectroscopy

The density matrix

Bloch sphere representation of quantum states

Introduction to multidimensional coherent spectroscopy

Concepts of multidimensional coherent spectroscopy

Coherent spectroscopy

Multidimensional coherent spectroscopy

Spectrum classification

Density matrix formalism and double-sided Feynman diagrams

Interpreting MDCS in the perturbative limit

Double-sided Feynman diagrams

Measured observables

Putting it all together

Case study: Two-level system

Phase matching

Two-dimensional infrared (2D IR) spectroscopy

Interpretation of multidimensional coherent spectra

Isolated two-level system

Inhomogeneously broadened ensemble of two-level systems

Gaussian inhomogeneity, constant homogeneous linewidth

Large inhomogeneity

Coherent coupling signatures

Incoherent coupling signatures

Doubly excited states and many-body interactions

Double-quantum spectra

Zero-quantum spectra

Three-dimensional coherent spectroscopy

Nonrephasing pathways and purely absorptive spectra

Finite-pulse effects

Mathematical formulations

Example spectra

Further applications

Experimental implementations

Experimental requirements and considerations

Precision and stability of time delays

Isolation of the signal

Detection of the signal

Overview of experimental approaches

Actively stabilized box geometry

Phase modulated collinear geometry

Comparison of different approaches

Data analysis

Multidimensional coherent spectroscopy of atomic ensembles.

Single- and zero-quantum 2D spectra of atomic vapors

MDCS in optically thick samples

Probing many-body interactions with double-quantum 2D spectroscopy

Probing many-body correlations with multi-quantum 2D spectroscopy

Frequency comb-based multidimensional coherent spectroscopy

Introduction to frequency combs and dual-comb spectroscopy

Frequency comb-based four-wave-mixing spectroscopy

Frequency comb-based single-quantum 2D spectroscopy

Frequency comb-based double-quantum 2D spectroscopy

Tri-comb spectroscopy

Two-dimensional spectroscopy of semiconductor quantum wells

Introduction to semiconductor optics

Many-body signatures in one-quantum 2D spectra

Many-body signatures in double- and multi-quantum 2D spectra

Two-dimensional spectroscopy of coupled quantum wells

Quantum well exciton-polaritons in microcavities

Fifth-order 3D infrared spectroscopy

Fifth-order 3D electronic spectroscopy

Third-order 3D electronic spectroscopy

Three-dimensional spectra of atomic vapors

Three-dimensional spectroscopy of semiconductor quantum wells

3D coherent spectroscopy of light-harvesting centers

3D coherent frequency domain spectroscopy

Two-dimensional spectroscopy of semiconductor quantum dots

Optical and electronic properties of quantum dots

2D coherent spectroscopy of GaAs quantum dots

2D spectroscopy of self-assembled In(Ga)As quantum dots

Coherent control of quantum dots

Coherent control within an ensemble of quantum dots

Coherent control of interactions between individual quantum dots

Two-dimensional spectroscopy of colloidal quantum dots

Two-dimensional spectroscopy of atomically thin 2D materials

Introduction to 2D materials

Homogeneous linewidth in 2D materials

Valley coherence and coupling in 2D materials.

Other applications of multi-dimensional coherent spectroscopy in Physics

Semiconducting carbon nanotubes

Color centers in diamond

Perovskite materials

New trends in multidimensional coherent spectroscopy

Broadening the spectral range: from terahertz to x-rays

THz MDCS

Improving the spatial resolution

Multidimensional spectroscopy with quantum light

Photoemission-detected MDCS

Figure Credits

References

Index

Blank Page

Blank Page.

Notes:

Description based on print version record.

Includes bibliographical references and index.

Other Format:

Print version: Li, Hebin Optical Multidimensional Coherent Spectroscopy

ISBN:

0-19-192649-3

0-19-265762-3

9780191926495

OCLC:

1257401588